Application of clay supported Gemini surfactants in triphase catalysis

CHED 946

Nahid Shabestary, nshabes@siue.edu, Timi J. Parker, timpark@siue.edu, and Neha H. Parikh, nparikh@siue.edu. Department of Chemistry, Southern Illinois University Edwardsville, Box 1652, Edwardsville, IL 62026-1652
We are using a naturally occurring clay mineral, hectorite (of the smectite family), to carry out intercalation reaction with dicationic quaternary ammonium Gemini surfactants. These novel, clay-supported catalysts will be used to study the kinetics of the SN2 displacement reaction converting n-butyl bromide to n-butyl chloride. Since Gemini surfactants are much more surface active than conventional surfactants containing a single cation (classical quaternary ammonium or phosphonium salts), it is interesting to see how they behave catalytically in a triphase system using toluene as the organic phase and water to dissolve the nuleophile. Triphase catalysis (TC) is a unique form of phase transfer catalysis (PTC) which greatly simplifies catalyst recovery and reuse. We have already synthesized several Gemini surfactants and developed clay supported catalysts for the triphase reaction.