Kinetics of synthesis of the ionic liquid 1-butyl-3-methylimidazolium bromide

PHYS 575

Jun Wang Sr., wangjun8828@zzuli.edu.cn, Xuzhao Yang Sr., xuzhao5378@sina.com, Gangsen Li Sr., lgs_chem@163.com, Zhenzhen Zhang, Yingying Shi, and Lihui Luan. College of Material Science and Chemical Engineering, Zhengzhou Uinversity of light industry, Dongfeng Road NO.5, zhengzhou, 450002, China
The kinetics of the synthesis of the ionic liquid 1-butyl-3-methylimidazolium bromide (IL) from1-methylimidazole (MIM) and 1-bromobutane (Br-Bu) in isopropyl alcohol as solvent were studied in a batchwise-operating stirred lab-scale glass reactor. The results show that the overall reaction was of second-order and the order of reaction for 1-methylimidazole and 1-bromobutane is first-order for each. The reaction rate constant at 323.15 K,328.15 K and 333.15 K is 0.0924 L•mol-1•h-1, 0.1692 L•mol-1•h-1 and 0.3228 L•mol-1•h-1,respectively. The apparent activation energy of the reaction between 1-methylimidazole and 1-bromobutane is 218 kJ•mol-1. Further, the reaction rate constant for 1-methylimidazole and bromoethane is 0.2926 L•mol-1•h-1 at 328.15 K, which indicated that the reaction rate of bromoethane with 1-methylimidazole was more fast than that of 1-bromobutane.