Study of gas-phase deposited lead sulfide nanocrystals embedded in oligomer matrices for optoelectronic devices

PHYS 190

Adam M. Zachary, azacha1@uic.edu, Igor L. Bolotin, bolotin@uic.edu, Daniel J. Asunskis, asunskis@uic.edu, Amanda T. Wroble, awrobl2@uic.edu, and Luke Hanley, lhanley@uic.edu. Department of Chemistry, University of Illinois at Chicago, MC 111, 845 W Taylor St, 4500 SES, Chicago, IL 60607
Lead sulfide nanocomposites are being examined for applications in photodetectors, light-emitting diodes, and photovoltaics. The optoelectronic properties of the composite can be tuned by varying the nanoparticle size and concentration within the organic matrix. Lead sulfide nanocomposite films are deposited with a modified commercial cluster beam deposition source. Transmission electron microscopy demonstrates that gaseous deposition can synthesize a composite film with <5 nm diameter lead sulfide nanocrystals of narrow size distribution embedded within either titanyl phthalocyanine or sexithiophene matrices. Nanocrystal inclusion increases the absorbance in the visible region compared to the organic matrix alone. X-ray photoelectron spectroscopy shows no oxidation or significant bonding between the nanocrystal and matrix. Nanocrystal formation via gaseous deposition displays advantages over traditional colloidal synthesis in the control of oxidation and particle density.
 

Nanostructured Materials
8:20 AM-12:00 PM, Tuesday, April 8, 2008 Morial Convention Center -- Rm. 338/339, Oral

Division of Physical Chemistry

The 235th ACS National Meeting, New Orleans, LA, April 6-10, 2008