Ring-substitution and the formation of polyaniline nanomaterials

CHED 285

Steve Da Silva and David M. Sarno, dsarno@qcc.cuny.edu. Department of Chemistry, Queensborough Community College - CUNY, 222-05 56th Avenue, Bayside, NY 11364
In recent years, polyaniline has been shown to be readily prepared as uniform nanofibers by simple synthetic procedures. We are investigating how ring-substitution on aniline influences nanoscale morphology. Electron microscopy has revealed that under the same conditions that yield polyaniline nanofibers, polymerization of methoxy-substituted o-anisidine yields only irregular clusters. Further, while methyl-substituted o-toluidine produces nanofibers from reactants at hundredth-molar concentrations, tenth molar concentrations yield microspheres with smooth surfaces and highly porous interiors. The variety of morphologies suggests that the molecular structure and conformation of the polymer play a significant role in the formation of these nanoscale materials.