Self-organization of porphyrins bearing hydrogen bonding motifs

INOR 267

Ivana Radivojevic, iradivojevic@gc.cuny.edu, Xinxu Shi, Sunaina Singh, and Charles Michael Drain, cdrain@hunter.cuny.edu. Department of Chemistry, Hunter College & Graduate Center of the City University of New York, 695 Park Avenue, New York City, NY 10021
Porphyrins bearing uracyl motifs at the four meso positions self-organize via homo complementary hydrogen bonds. The morphology of the materials found by deposition of 5,10,15,20 – tetrakis (1-butyl-6-uracyl) porphyrinato Zn(II) (TUrZnP) depends on a verity of environmental conditions. For example, atomic force microscopy (AFM) measurements reveal that 10 µM solutions in "wet" THF onto mica and glass results in thin films (5-20 nm thick), whereas deposition from "dry" THF yields nanofibers and nanorods on mica and glass. The variables that influence the morphology of the deposit material will be presented. These materials were further characterized by fluorescence microscopy and UV-Vis absorption spectroscopy. The investigation of these nanoscopic materials is relevant to solar energy harvesting in terms of self-organized antenna complex found in chlorophyll molecules in nature.
 

Nanoscience: Applications
7:00 PM-10:00 PM, Sunday, August 19, 2007 BCEC -- Exhibit Hall - B2, Poster

Division of Inorganic Chemistry

The 234th ACS National Meeting, Boston, MA, August 19-23, 2007