Synthesis of vanadium(III) cage clusters for catalytic use

INOR 389

Andrew W. Scott, awscott@ilstu.edu, Michael P. Weberski Jr., mpweber@ilstu.edu, and Craig C. McLauchlan, mclauchlan@ilstu.edu. Department of Chemistry, Illinois State University, CB 4160, Normal, IL 61790-4160
Vanadium coordination complexes have been found to have many practical uses including catalytic oxidation. It is known that an extended material with the formula VOPO4 can be used as a catalyst in formation of maleic anhydride. The goal of our research is to make a discrete molecular structure of the general formula V4P4O12R4R4', “{VOPO3}4”, which has a cube-like structure and contains a V(III) with an octahedral coordination environment. The cube-like structure is thought to have a larger surface area, which will increase catalytic ability. These complexes are characterized via X-ray crystallography, NMR, EPR, IR, UV-Vis, and magnetic susceptibility. Here we report our recent results with the {VOPO3}4 cages, including a recent X-ray structure characterization.
 

5th International Symposium on Chemistry and Biological Chemistry of Vanadium: Posters in Chemistry and Biochemistry
7:00 PM-10:00 PM, Sunday, 10 September 2006 Moscone Center -- Hall D, Poster

Sci-Mix
8:00 PM-10:00 PM, Monday, 11 September 2006 Moscone Center -- Hall D, Sci-Mix

Division of Inorganic Chemistry

The 232nd ACS National Meeting, San Francisco, CA, September 10-14, 2006