Synthesis, structure and surface photovoltage property of a 3D Ni (II) coordination polymer

INOR 161

Shu Yun Niu, syniu@sohu.com, Li Ping Sun, syniu@sohu.com, and Jing Jin. School of Chemistry and Chemical Engineering, Liaoning Normal University, Huanghe Road 850, Dalian, 116029, China
A novel 3D infinite coordination polymer [Ni2(HCOO) 4(H2O)4]n has been synthesized and characterized by single crystal X-Ray diffraction. In crystal there are two crystallo-graphically independent Ni(II) ions. Ni1 is coordinated by six HCOO groups and Ni2 is coordinated by two HCOOand four water molecules. HCOO link the Ni1 to form a 2D layer. Ni2 lie among the 2D layers and connect with the layer by the HCOO, which makes the 2D layers into 3D network. The SPS of complex indicate that there are four positive SPV responses at 300-800nm. The responses at 331nm and 346nm are separately be assigned to the pp* charge transfer transition and LMCT transition. The responses at 397nm and 644nm are attributed to the d →d* transition of Ni(II), which are separately 3A2g3T1g and 3A2g3T2g. This work was supported by the NSFC (Nos. 20571037 and 90201018 )
 

Coordination Chemistry: Characterization and Applications
7:00 PM-10:00 PM, Sunday, 10 September 2006 Moscone Center -- Hall D, Poster

Sci-Mix
8:00 PM-10:00 PM, Monday, 11 September 2006 Moscone Center -- Hall D, Sci-Mix

Division of Inorganic Chemistry

The 232nd ACS National Meeting, San Francisco, CA, September 10-14, 2006