Computational studies on uranyl complexes in aqueous solution

INOR 906

Notker Roesch, roesch@ch.tum.de, Florian Schlosser, Sven Krueger, Lyudmila V. Moskaleva, and Alexei V. Matveev. Theoretische Chemie, TU Muenchen, Lichtenbergstrasse 4, 85748 Garching, Germany
Relativistic all-electron density functional calculations have been performed on various uranyl complexes that occur in natural aqueous systems. Mononuclear as well as bi- and trinuclear carbonato complexes are compared. The reduced stability of the triuranyl-hexacarbonato complex compared to mononuclear species is rationalized by an effective undercoordination of the uranyl moieties, which is supported by geometry and energy data. In agreement with experiment, various isomers of uranyl-hydroxo-carbonate are found to be nearly degenerate. Also fundamental thermochemical data for uranyl are discussed and an accurate value for the enthalpy of formation of uranyl is derived.
 

Computational Chemistry
8:30 AM-12:10 PM, Wednesday, 13 September 2006 Moscone Center -- Room 305, Oral

Division of Inorganic Chemistry

The 232nd ACS National Meeting, San Francisco, CA, September 10-14, 2006