Treatment of atrazine-contaminated water by Ni/Fe bimetallic system

ENVR 166

Shao-ping Tong, sptong@zjut.edu.cn1, Wei-ping Liu, toptong@eyou.com2, and Chun-an Ma1. (1) College of Chemical Engineering and Materials Science, Zhejiang University of Technology, Caohuang Road, Hangzhou, 310032, China, (2) Researching Centre of Environmental Science, Zhejiang University of Technology, Caohuang Road, Hangzhou, 310032, China
Degradation of atrazine via its reaction with Ni/Fe powder was conducted in aqueous solution. The experimental results showed that Ni/Fe had great catalytic activity on the treatment of atrazine-contaminated water and the dechlorination efficiency was dependent on both the amount of Ni loading on Fe's surface and pH values of the solution. The catalyst of 2.95% Ni/Fe had the largest surface area and was the optimum proportion for atrazine dechlorination. Catalytic activity of Ni/Fe was very obvious only when the pH value of the solution was less than 4.0. The reaction approximately followed first-order kinetics under the experimental conditions, and the apparent rate constants at pH=2.0, 3.0 and 4.0 were 0.07518, 0.06212 and 0.00131min-1, respectively. The electrochemical measurements showed the adsorbed hydrogen must be the dominating reducing agent for atrazine dechlorination in water.
 

General Papers
6:00 PM-8:00 PM, Wednesday, 13 September 2006 Moscone Center -- Hall D, Poster

Division of Environmental Chemistry

The 232nd ACS National Meeting, San Francisco, CA, September 10-14, 2006