Future prospects for fully coherent vibrational and electronic spectroscopy in analytical chemistry

ANYL 229

John C. Wright, Wright@chem.wisc.edu, Andrei V. Pakoulov, Mark A. Rickard, marickard@wisc.edu, Kathryn M. Kornau, kornau@chem.wisc.edu, and Nathan A. Mathew, mathew@chem.wisc.edu. Department of Chemistry, University of Wisconsin, 1101 University Avenue, Madison, WI 53706
Absorption and fluorescence spectroscopy is based on changing the populations of different quantum states. Quenching destroys excited state populations and limits fluorescence methods to molecules with low quenching rates. A new family of fully coherent spectroscopies has been developed that are based on creating coherent entanglements of quantum states that emit intensely in directional beams that can be easily measured. Unlike populations, coherences are like those responsible for refraction and NMR- their emission cannot be quenched. A particularly interesting capability is the creation of the same multiple- and zero- quantum coherences used in NMR. In this talk, we demonstrate all possible coherent spectroscopies using three beams including the CT3 and HMQC' methods proposed by Mukamel. We show that the methods are inherently 6-dimensional experiments and allow one to apply coherent multidimensional spectroscopy to the wide range of quantum states of interest in science.