Amphiphilic conetworks comprising a fluorophilic phase

POLY 442

Nico Bruns, nico.bruns@fmf.uni-freiburg.de, Freiburg Materials Research Center, University of Freiburg, Stefan-Meier-Str. 21, 79104 Freiburg, Germany and Joerg C. Tiller, joerg.tiller@fmf.uni-freiburg.de, Institute for Macromolecular Chemistry and Freiburg Materials Research Center, University of Freiburg, Stefan-Meier-Str. 21, 79104 Freiburg, Germany.
Amphiphilic conetworks, generally considered as hydrophilic/hydrophobic materials, are recently gaining great interest due their wide range of possible applications in catalysis, sensors, and biomedical applications. However, little is known about conetworks with highly fluorinated phases. Here, we describe two readily available methods that allow the synthesis of nanophase separated hydrophobic/fluorophilic and hydrophilic/fluorophilic conetworks. The potential of the hydrophilic/fluorophilic conetworks as phase transfer matrix for reactions in supercritical CO2, was examine by loading the conetworks with lipase from Rhizomucor miehei. These systems showed an increased activity of the enzyme in supercritical CO2 by a factor of 42 compared to conventional enzyme powder.
 

Biocatalysis in Polymer Science
6:00 PM-8:00 PM, Tuesday, 12 September 2006 Moscone Center -- Hall D, Poster

Sci-Mix
8:00 PM-10:00 PM, Monday, 11 September 2006 Moscone Center -- Hall D, Sci-Mix

Division of Polymer Chemistry

The 232nd ACS National Meeting, San Francisco, CA, September 10-14, 2006