Multifunctional coatings based on chemical vapor depostion co-polymerization

POLY 78

Joerg Lahann, lahann@umich.edu, Hsien-Yeh Chen, hsienyc@umich.edu, and Yaseen Elkasabi. Department of Chemical Engineering, Materials Science and Engineering, and Macromolecular Science and Engineering, University of Michigan, 2300 Hayward Street, GGBL 3414, Ann Arbor, MI 48105
The controlled and stable immobilization of one or multiple types of (bio)molecules to a surface has been identified as one of the critical challenge in the areas of biochips and biosensors. Using chemical vapor deposition co-polymerization, we have developed a simple strategy towards multi-functional surfaces presenting two different biological ligands in controllable ratios. For CVD co-polymerization, mixtures of 4-trifluoroacetyl [2.2]paracyclophane and 4-aminomethyl [2.2]paracyclophane were sublimated, converted to the corresponding quinodimethanes (monomers) and co-polymerized onto the substrate. CVD co-polymerization of 1 and 2 resulted in transparent and topologically uniform polymer films with functional groups in controllable ratios. All polymer films are characterized by X-ray photoelectron spectroscopy, infrared spectroscopy, X-Ray diffraction analysis, imaging ellipsometry and fluorescence imaging (after binding). These modularly designable polymer coatings are applicable to a wide range of biomedical devices including microanalytical or diagnostic systems.
 

Polymers in Biosensors and Biochips
1:30 PM-4:40 PM, Sunday, 10 September 2006 San Francisco Marriott -- Salon 12/13, Oral

Division of Polymer Chemistry

The 232nd ACS National Meeting, San Francisco, CA, September 10-14, 2006